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---Mr Smith spent as much time as he ________ the experiments．
---No doubt he succeeded in the end．

A.
could do
B.
could to do
C.
could doing
D.
could on doing

C
解析：
本題涉及到spend time(in)doing sth．和as much…as one can結構．

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---Mr Smith spent as much time as he ________ the experiments．---No doubt he succeeded in the end．

We are going to have a picnic this coming weekend. Would you ________ us, Mr. Smith?

---Mr Smith spent as much time as he ________ the experiments．
---No doubt he succeeded in the end．